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I tried to do this last night. It was tough! I learned a few things. When I learned that when I concentrate my face changes. Then when the girl sees me she quickly looks away.
I never got a hi or a smile back. From a distance I got bad looks and up close girls looked away. But I am going to try again next sat, during the day.
It's hard to tell exactly what you're talking about, but it sounds like you may have just been looking around staring and smiling at girls. In my opinion I don't think you should smile at a girl until you've had a few separate sets of eye contact or a few solid seconds of it. If a girl just happens to catch your eye, and you're smiling already or do it immediately, it could come off as a bit creepy. Be sure she gives you the IOI of multiple eye contacts before returning one with a smile.