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Jack's reply has merit. If you could get her invested in you, for instance be able to do something no other guy can, she is more likely to give you a chance.
This is the careful line that you have to walk because that leads to over-the-top behavior. I'm more of a fan of just creating an emotional spark/emotional tension. Most women have felt certain emotions when they've met a guy that they like and they will go on autopilot if those emotions are triggered again then they will react in the same manner. The real point that I was trying to get at is to make an effort to remove time as an obstacle. More time in the initial meeting. Less time between the initial meeting and walking away. So I wouldn't go for doing something that no other guy can do and instead of that doing what other guys have done to make themselves attractive to her. Usually, that is simply making her feel better about herself when she's around you.